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Nonlinear quantum interferometric spectroscopy with entangled photon pairs

delete2022-03-03
delete11
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OA
AI
S
Shahaf Asban
V
Vladimir Chernyak
S
Shaul Mukamel *
DOI:10.1063/5.0079049delete
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Abstract

Abstract

En 中文
We develop closed expressions for a time-resolved photon counting signal induced by an entangled photon pair in an interferometric spectroscopy setup. Superoperator expressions in Liouville-space are derived that can account for relaxation and dephasing induced by coupling to a bath. Interferometric setups mix matter and light variables non-trivially, which complicates their interpretation. We provide an intuitive modular framework for this setup that simplifies its description. Based on the separation between the detection stage and the light-matter interaction processes, we show that the pair entanglement time and the interferometric time-variables control the observed physics time scale. Only a few processes contribute in the limiting case of small entanglement time with respect to the sample response, and specific contributions can be singled out. Published under an exclusive license by AIP Publishing.
Keywords:
COHERENCE
NANOSTRUCTURES
INFORMATION
PARAMETERS
EXCITONS
LIGHT

Journal

Journal of Chemical Physics cover
Journal of Chemical Physics
IF:
3.1
Papers:
7.2W
Citations:
23.2W

Organization

University of California System cover
University of California System
Scholars:
37.2W
Papers: 33.6W
Citations: 6.6K
U
university of california irvine
Scholars:
2.2W
Papers: 1.7W
Citations: 55