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Probing Non-Equilibrium Pair-Breaking and Quasiparticle Dynamics in Nb Superconducting Resonators Under Magnetic Fields

delete2025-01-27
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OA
AI
J
J.-M. Park
Z
Zhi Xiang Chong
R
Richard H. J. Kim
S
Samuel Haeuser
R
R. K. Chan
A
Akshay A. Murthy
C
Cameron Kopas
J
Jayss Marshall
E
Ella Lachman
J
J. Mutus
A
Anna Grassellino
A
Alex Romanenko
J
Jigang Wang *
DOI:10.3390/ma18030569delete
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Abstract

Abstract

En 中文
We conducted a comprehensive study of the non-equilibrium dynamics of Cooper pair breaking, quasiparticle (QP) generation, and relaxation in niobium (Nb) cut from superconducting radio-frequency (SRF) cavities, as well as various Nb resonator films from transmon qubits. Using ultrafast pump-probe spectroscopy, we were able to isolate the superconducting coherence and pair-breaking responses. Our results reveal both similarities and notable differences in the temperature- and magnetic-field-dependent dynamics of the SRF cavity and thin-film resonator samples. Moreover, femtosecond-resolved QP generation and relaxation under an applied magnetic field reveals a clear correlation between non-equilibrium QPs and the quality factor of resonators fabricated by using different deposition methods, such as DC sputtering and high-power impulse magnetron sputtering. These findings highlight the pivotal influence of fabrication techniques on the coherence and performance of Nb-based quantum devices, which are vital for applications in superconducting qubits and high-energy superconducting radio-frequency applications.
Keywords:
ultrafast pump-probe
superconductivity
superconducting quantum computer
non-equilibrium quasiparticles
superconducting radio frequency (SRF)
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Materials
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3.2
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Iowa State University
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Ames National Laboratory
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united states department of energy (doe)
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