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Process swing adsorption with selective purge gas recirculation (PSA-SPUR): unlocking CO2 capture from flue gas via Zr-MOF adsorbents
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DOI：10.1016/j.ceja.2026.101259.png)
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Abstract
En 中文
• UiO-66-(OH)₂ achieves 91 CO₂/N₂ IAST selectivity and 1.96 mmol g⁻¹ working capacity at 0.15 bar. • PSA-SPUR process theoretically enables both 100% CO₂ recovery/purity from 15% flue gas at moderate vacuum (≥0.15 bar). • Synergy between MOF adsorbent and process design drastically enhances the performance of CO2 capture PSA systems.
Keywords:
Carbon capture
Pressure swing adsorption
Selective purge gas recirculation
MOF
Equilibrium Theory
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