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Programmable hydrogels by combining persistent and transient dynamic bonds
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DOI：10.1016/j.cej.2026.174743.png)
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Abstract
En 中文
• Dynamic hydrogel networks that respond to chemical fuels were developed • Two orthogonal linkers were included, dynamic but persistent metal-ligand coordination and temporally controlled anhydrides • Addition of carbodiimide fuel enhanced modulus transiently, while material retained dynamic properties • Complex patterns of mechanical properties could be temporally programmed and the materials showed good self-healing
Keywords:
Dynamic hydrogels
Programmable materials
Metal-ligand coordination
Anhydride linkers
Self-healing properties
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