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Recent Advances in Developing High-Performance Solid-State Lithium Batteries: Interface Engineering
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DOI：10.1021/acs.energyfuels.3c01626.png)
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Abstract
En 中文
Tosurmount constraints, the increasing demand for electric vehiclesand networks necessitates the use of lithium-ion batteries (LIBs)that traditionally use electrolytes that are volatile organic liquids(LEs). Increasing demand for electric networks and automobiles necessitatessafer batteries in the presence of more energy. Lithium solid-statebatteries (SSBs) have recently gained popularity as alternatives toLEs. However, the interface instability between solid electrolytes(SEs) and electrodes limits the energy density of SSBs. With parasiticreactions and dendrite growth, this culminates in a short cycle lifeand a dissatisfied coulombic efficiency. Significant advancementshave been made in the field of SEs. Nevertheless, substantial challengesstill exist that prevent the practical use of SSBs with high energydensities. This review summarizes the most current findings in thestudy of electrolytes. Basic comprehension of the mechanism, scientificobstacles, and solutions to electrolyte limitations for high-performanceSSBs are covered. Numerous strategies for addressing interface issuesare analyzed, and as a result, some recommendations are made regardingthe optimal electrolyte characteristics for practical applications.At the end of this review, key concerns and proposals for future studyinto how best to develop high-performance lithium SSBs are discussed.
Keywords:
HIGH-ENERGY DENSITY
ATOMIC LAYER DEPOSITION
PULSED-LASER DEPOSITION
LI-METAL
GARNET ELECTROLYTE
COMPOSITE ANODE
ION BATTERIES
RESISTANCE
SURFACE
ORIGIN