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Reinforced 1D perovskite growth via molecular synergy for enhanced perovskite solar cells stability

delete2026-08-11
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PRE
AI
Z
Zhixu Zhou
Z
Zhe Li
Y
Yue Zang *
Y
Yibo Tu
W
Weihong Liu
Z
Zhikang Zhu
W
Wensheng Yan *
DOI:10.1016/j.cej.2026.180548delete
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Abstract

Abstract

En 中文
• A choline chloride–sulfamide (CSR) synergistic bimolecular engineering is developed to precisely regulate 1D perovskite growth on 3D perovskite surfaces for inverted solar cells. • Bimolecular interaction and defect passivation facilitate oriented 1D perovskite formation, eliminate residual PbI2, and refine energy level alignment. • The CSR-modified inverted perovskite solar cell achieves a champion efficiency of 25.30% with simultaneously improved VOC and fill factor. • Multifunctional interfacial engineering suppresses non-radiative recombination and enhances charge extraction at the perovskite/ETL interface. • The device exhibits outstanding stability, retaining 82.01% efficiency after 500 h thermal aging and 86% after 800 h MPP tracking.
Keywords:
Perovskite solar cells
One-dimensional perovskite
Synergistic interaction
Ion exchange
Interface engineering)

Journal

Chemical Engineering Journal cover
Chemical Engineering Journal
IF:
13.2
Papers:
7.2W
Citations:
48.5W

Organization

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