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Single atom visibility in STEM optical depth sectioning

delete2016-10-19
delete42
PRE
AI
R
Ryo Ishikawa *
S
Stephen J. Pennycook
A
Andrew R. Lupini
S
Scott D. Findlay
N
Naoya Shibata
Y
Yuichi Ikuhara
DOI:10.1063/1.4965709delete
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Abstract

Abstract

En 中文
The continuing development of aberration correctors for the scanning transmission electron microscope (STEM) offers the possibility of locating single atoms in crystals in 3D via optical depth sectioning. The main factors that determine the feasibility of such an approach are visibility and dose requirements. Here, we show how Poisson's statistics can be quantitatively incorporated into STEM image simulations and demonstrate that the 3D location of single cerium atoms in wurtzite-type aluminum nitride is indeed feasible under large-angle illumination conditions with a relatively low dose. We also show that chromatic aberration does not presently represent a limitation provided a cold field emission source is used. These results suggest efforts into improved aberration corrector designs for larger illumination angles that offer significant potential for 3D structure determination of materials. Published by AIP Publishing.
Keywords:
CONFOCAL ELECTRON-MICROSCOPY
ABERRATION
RESOLUTION
DOPANT
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Journal

Applied Physics Letters cover
Applied Physics Letters
IF:
3.6
Papers:
10.4W
Citations:
17.8W

Organization

U
University of Tokyo
Scholars:
7.1W
Papers: 6.5W
Citations: 2.2K
U
united states department of energy (doe)
Scholars:
11.3W
Papers: 9.6W
Citations: 246
N
National University of Singapore
Scholars:
7.5W
Papers: 6.5W
Citations: 11.4W
O
oak ridge national laboratory
Scholars:
1.4W
Papers: 1.0W
Citations: 20
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