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Tailoring the nature of zirconium sites on support to maximize catalytic upgrading of furfural
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OA
AI
Z
J
C
J
G
X
刘
丁
DOI：10.1016/j.mcat.2026.116247.png)
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Abstract
En 中文
• ZrOx/CB enhances the MPV hydrogenation of furfural to selectively produce furfuryl alcohol. • Zr/Me-BEA facilitates the tandem hydrogenation–etherification reaction to alkyl furfuryl ether. • Isolated ZrOH hydrogen-bonded with SiOH groups within zeolite pores serve as the Lewis acidic active sites. • Surface functionalities on support determine the nature of Zr active sites and thus dominate the catalytic reaction pathways.
Keywords:
Furfural
Transfer hydrogenation
Etherification
Hierarchical zeolites
Zirconium sites
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