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Tuning chain mobility and anisotropic ion transport in composite polymer electrolytes via short-chain polyethylene oxide surface modification
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DOI：10.1016/j.jtice.2026.106895.png)
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Abstract
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• MD data reveal anisotropic Li transport at LATP/PEO electrolyte interfaces. • Pristine LATP induces polymer layering that restricts Li to 2D motion. • Short-chain PEO modifications disrupt ordering to enable 3D Li conduction. • 25% modification shows optimal interfacial impedance reduction of nearly 60%. • Excessive modification hinders ion transport due to steric crowding.
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