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Unlocking high-efficiency electrosynthesis of N,N-dimethylformamide through the synergy of three-dimensional ordered macroporous superstructure and implanted nano-tentacles

delete2025-09-18
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PRE
AI
Y
Yingchun He
X
Xin Xiao
X
Xiaofang Li
D
Dong-Dong Ma
Q
Qiang Xu *
朱起龙 (Qi‐Long Zhu) *
DOI:10.1016/j.apcatb.2025.125989delete
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Abstract

Abstract

En 中文
• An ordered macroporous superstructure decorated with nano-tentacles has been elaborately designed and synthesized. • The electrosynthesis of N,N-dimethylformamide achieves 44 % Faradaic efficiency and 325 μmol h–1 cm–2 productivity. • In situ characterization combined with DFT calculations provide a comprehensive understanding of the reaction mechanism. • Finite element analysis highlights the pronounced tip-intensified effect of the nano-tentacles in the catalyst.

Journal

A
Applied Catalysis B Environment and Energy
IF:
21.1
Papers:
4.2K
Citations:
18.2W

Organization

F
Fujian Institute of Research on the Structure of Matter
Scholars:
660
Papers: 221
Citations: 1.7W
S
Southern University of Science and Technology
Scholars:
5.2K
Papers: 2.1K
Citations: 34
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