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Unraveling gas–surface combined mechanism in ethane catalytic partial oxidation over nickel catalysts via experiment and microkinetic modeling
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DOI：10.1016/j.jcat.2026.117100.png)
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Abstract
En 中文
• SVUV-PIMS detects key radicals (C2H5, C3H3, aC3H5) in ethane CPO. • Coupled microkinetic model captures gas–surface chemistry interplay. • Surface dehydrogenation dominates while H-abstraction is rate-determining. • Competing oxidative cracking and coupling kinetics are quantitively revealed. • C3 radicals reveal pathway to aromatics and coke precursors.
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6.5
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1.2W
Citations:
5.1W
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